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Fehn, Professor of Geology
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Fumaroles and crater lake, White Island, New Zealand
Background:
Cosmogenic isotopes derive their name from the fact that they are formed
as a consequence of the interaction of cosmic rays with atoms of the
atmosphere, hydrosphere, or the top layers of the lithosphere. Although
the group includes stable isotopes such as 3He, most of the
isotopes in question are radioactive. Commonly we refer to 10Be,
14C, 26Al, 36Cl, 41Ca and
129I as part of this group. In spite of their commonly
used name, most of these isotopes are also produced by processes other
than interaction with cosmic rays; in particular, nuclear reactions
in the crust and the anthropogenic nuclear activities have added significantly
to the total concentrations of these isotopes. Because these isotopes
have generally very low concentrations and relatively long half-lives
with correspondingly low levels of radioactivity, they cannot (with
the exception of 14C) be measured with methods such as conventional
mass spectrometry or counting techniques. The development of accelerator
mass spectrometry (AMS) has made the detection of these isotopes at
the low natural levels possible, and has opened up a wide field of applications,
in areas such as hydrogeology, oceanography, geomorphology, and
volcanology.
The release into the environment of some of these isotopes from
nuclear explosions and reprocessing has also made possible applications
of these isotopes in environmental studies and in short-term geologic
questions.
At the Cosmogenic Isotope Laboratory, we have used mainly two of these
isotopes, 129I and 36Cl, which have half-lives
of 15.7 Ma and 301 ka, respectively. We have used these isotopes
particularly in the tracing and dating of aquifers (Fehn et al.,1992;
Rao et al., 1996), of fluids associated with hydrocarbons (Fehn et al.,
1990; Moran et al.,1995) and of organic material in marine sediments
(Moran et al., 1998). Samples are prepared at our laboratory and sent
for analysis to the PRIME Laboratory at Purdue University.
Iodine-129 is derived
from cosmogenic, natural fissiogenic, and anthropogenic sources.
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